Litcius/Paper detail

Copper‐Catalyzed and Proton‐Directed Selective Hydroxymethylation of Alkynes with CO<sub>2</sub>

Mei‐Yan Wang, Xin Jin, Xiaofei Wang, Shumei Xia, Yue Wang, Shouying Huang, Ying Li, Liang‐Nian He, Xinbin Ma

2020Angewandte Chemie International Edition47 citationsDOI

Abstract

Abstract An intriguing strategy for copper‐catalyzed hydroxymethylation of alkynes with CO 2 and hydrosilane was developed. Switched on/off a proton source, for example, t BuOH, direct hydroxymethylation and reductive hydroxymethylation could be triggered selectively, delivering a series of allylic alcohols and homobenzylic alcohols, respectively, with high levels of Z / E , regio‐ and enantioselectivity. Such a selective synthesis is attributed to the differences in response of vinylcopper intermediate to proton and CO 2 . The protonation of vinylcopper species is demonstrated to be prior to hydroxymethylation, thus allowing a diversion from direct alkyne hydroxymethylation to reductive hydroxymethylation in the presence of suitable proton.

Topics & Concepts

Allylic rearrangementProtonationCatalysisChemistryProtonAlkyneMedicinal chemistryCombinatorial chemistryCopperOrganic chemistryPhysicsQuantum mechanicsIonCarbon dioxide utilization in catalysisAsymmetric Hydrogenation and CatalysisCO2 Reduction Techniques and Catalysts