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Orbital Diffusion, Polarization, and Swapping in Centrosymmetric Metals

Xiaobai Ning, Armando Pezo, Kyoung‐Whan Kim, Wang Kang, Kyung‐Jin Lee, Aurélien Manchon

2025Physical Review Letters12 citationsDOIOpen Access PDF

Abstract

We propose a general theory of charge, spin, and orbital diffusion based on Keldysh formalism. Our findings indicate that the diffusivity of orbital angular momentum in metals is much lower than that of spin or charge due to the strong orbital intermixing in crystals. Furthermore, our theory introduces the concept of "spin-orbit polarization" by which a pure orbital (spin) current induces a longitudinal spin (orbital) current, a process as efficient as spin polarization in ferromagnets. Finally, we find that orbital currents undergo momentum swapping, even in the absence of spin-orbit coupling. This theory establishes several key parameters for orbital transport of direct importance to experiments.

Topics & Concepts

Polarization (electrochemistry)Materials scienceDiffusionCondensed matter physicsChemical physicsPhysicsQuantum mechanicsPhysical chemistryChemistryQuasicrystal Structures and PropertiesRare-earth and actinide compoundsMagnetic properties of thin films
Orbital Diffusion, Polarization, and Swapping in Centrosymmetric Metals | Litcius