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Synthesis of Trifluoromethyl- and Ester Group-Substituted α-Carbolines via Iron-Catalyzed Tandem Cyclization Reaction

Yumin Xu, Xiaoqian Chen, Yiqin Gao, Zicong Yan, Changfeng Wan, Jin‐Biao Liu, Zhiyong Wang

2020The Journal of Organic Chemistry20 citationsDOI

Abstract

An efficient approach to prepare trifluoromethyl-α-carbolines and ester group-substituted α-carbolines via the tandem cyclization reaction of 2-(2-aminophenyl)acetonitriles and trifluoromethyl 1,3-diones or β,γ-unsaturated α-ketoesters was reported. The transformation proceeded smoothly in the presence of catalytic environmental-benign iron salts, which are used to prepare the desired products in moderate to good yields.

Topics & Concepts

ChemistryTrifluoromethylAcetonitrilesTandemCatalysisGroup (periodic table)Medicinal chemistryOrganic chemistryCombinatorial chemistryAcetonitrileAlkylMaterials scienceComposite materialFluorine in Organic ChemistryAsymmetric Synthesis and CatalysisCatalytic C–H Functionalization Methods
Synthesis of Trifluoromethyl- and Ester Group-Substituted α-Carbolines via Iron-Catalyzed Tandem Cyclization Reaction | Litcius