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Nonlinear Electronic Density Response in Warm Dense Matter

Tobias Dornheim, Jan Vorberger, M. Bönitz

2020Physical Review Letters85 citationsDOIOpen Access PDF

Abstract

Warm dense matter (WDM)-an extreme state with high temperatures and densities that occurs, e.g., in astrophysical objects-constitutes one of the most active fields in plasma physics and materials science. These conditions can be realized in the lab by shock compression or laser excitation, and the most accurate experimental diagnostics is achieved with lasers and free electron lasers which is theoretically modeled using linear response theory. Here, we present first ab initio path integral Monte Carlo results for the nonlinear density response of correlated electrons in WDM and show that for many situations of experimental relevance nonlinear effects cannot be neglected.

Topics & Concepts

Warm dense matterPhysicsPath integral Monte CarloNonlinear systemPlasmaElectronLaserExcitationComputational physicsAb initioState of matterMonte Carlo methodStatistical physicsPath integral formulationQuantum mechanicsQuantumMathematicsStatisticsHigh-pressure geophysics and materialsAdvanced Chemical Physics StudiesLaser-induced spectroscopy and plasma
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