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Electrochemical selective divergent C–H chalcogenocyanation of <i>N</i>-heterocyclic scaffolds

Kusum Ucheniya, Pooja Kumari Jat, Amreen Chouhan, Lalit Yadav, Satpal Singh Badsara

2024Organic & Biomolecular Chemistry11 citationsDOI

Abstract

]quinolines were also successfully chalcogenocyanated under the optimized reaction conditions providing a platform for the synthesis of pharmaceutically privileged molecules. By switching the reaction conditions, the developed protocol offers selective synthesis of C-3 thiocyanate and 1,3 bis-thiocyanate indolizines in good to excellent yields under catalyst-free conditions. On the basis of control experiments and cyclic voltammetry data, a plausible reaction pathway is also presented.

Topics & Concepts

IndolizineChromoneElectrochemistryChemistryEnonePolar effectCombinatorial chemistryMedicinal chemistryStereochemistryElectrodePhysical chemistryCatalytic C–H Functionalization MethodsRadical Photochemical ReactionsSynthesis and Reactivity of Heterocycles
Electrochemical selective divergent C–H chalcogenocyanation of <i>N</i>-heterocyclic scaffolds | Litcius