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Magnetic and electronic phase transitions probed by nanomechanical resonators

Makars Šiškins, Martin Lee, Samuel Mañas‐Valero, Eugenio Coronado, Yaroslav M. Blanter, Herre S. J. van der Zant, Peter G. Steeneken

2020Nature Communications108 citationsDOIOpen Access PDF

Abstract

Abstract The reduced dimensionality of two-dimensional (2D) materials results in characteristic types of magnetically and electronically ordered phases. However, only few methods are available to study this order, in particular in ultrathin insulating antiferromagnets that couple weakly to magnetic and electronic probes. Here, we demonstrate that phase transitions in thin membranes of 2D antiferromagnetic FePS 3 , MnPS 3 and NiPS 3 can be probed mechanically via the temperature-dependent resonance frequency and quality factor. The observed relation between mechanical motion and antiferromagnetic order is shown to be mediated by the specific heat and reveals a strong dependence of the Néel temperature of FePS 3 on electrostatically induced strain. The methodology is not restricted to magnetic order, as we demonstrate by probing an electronic charge-density-wave phase in 2H-TaS 2 . It thus offers the potential to characterize phase transitions in a wide variety of materials, including those that are antiferromagnetic, insulating or so thin that conventional bulk characterization methods become unsuitable.

Topics & Concepts

Condensed matter physicsPhase transitionvan der Waals forceAntiferromagnetismMaterials scienceFerromagnetismPhase (matter)PhysicsQuantum mechanicsMolecule2D Materials and ApplicationsTopological Materials and PhenomenaMechanical and Optical Resonators