Litcius/Paper detail

Asymmetric Allylation by Chiral Organocatalyst‐Promoted Formal Hetero‐Ene Reactions of Alkylgold Intermediates

Guizhi Dong, Ming Bao, Xiongda Xie, Shi‐Kun Jia, Wenhao Hu, Xinfang Xu

2020Angewandte Chemie International Edition55 citationsDOI

Abstract

An unprecedented catalytic asymmetric allylation of isatins and isatin-derived ketimines is reported enabled by a gold and chiral organocatalyst cooperative catalysis strategy. This method offers expeditious access to chiral 2,5-disubsituted alkylideneoxazolines containing vicinal stereogenic centers, mainly in optically pure form, and which are otherwise impossible to access. Mechanistic evidence reveals the presence of an alkylgold intermediate, and an X-ray crystal structure of the allylgold species illuminates its unique stability and reactivity. An asymmetric formal hetero-ene reaction of this gold intermediate, involving a dearomatization process, is enabled with assistance of a quinine-derived squaramide catalyst. This novel discovery extends the synthetic applications of gold complexes and the versatility of gold catalysis.

Topics & Concepts

StereocenterChemistryEnantioselective synthesisCatalysisSquaramideCombinatorial chemistryEne reactionVicinalIsatinReactivity (psychology)Nitroaldol reactionOrganocatalysisOrganic chemistryPathologyMedicineAlternative medicineCatalytic Alkyne ReactionsCatalytic C–H Functionalization MethodsAsymmetric Synthesis and Catalysis