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Puncture-resistant self-healing polymers with multi-cycle adhesion and rapid healability

Bingrui Li, Sirui Ge, Sheng Zhao, Kunyue Xing, Alexei P. Sokolov, Pengfei Cao, Tomonori Saito

2023Materials Horizons22 citationsDOIOpen Access PDF

Abstract

. U-PDMS-SPs exhibit fast autonomous self-healability with 25% strain recovery within 2 minutes of healing, and over 90% toughness recovery after 16 hours. We further demonstrate its puncture-resistant properties under the ASTM D5748 standard with an unbreakable feature. Furthermore, the multi-cycle adhesive properties of U-PDMS-SPs are also revealed. High puncture resistance (>327 mJ) and facile adhesion with rapid autonomous self-healability will have a broad impact on the design of adhesives, roofing materials, and many other functional materials with enhanced longevity.

Topics & Concepts

Self-healingAdhesionMaterials sciencePolymerSelf-healing materialNanotechnologyBiomedical engineeringMedicineComposite materialPathologyAlternative medicinePolymer composites and self-healingAdvanced Polymer Synthesis and CharacterizationPhotopolymerization techniques and applications
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