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Electron-phonon coupling and competing Kekulé orders in twisted bilayer graphene

Yves H. Kwan, Glenn Wagner, Nick Bultinck, Steven H. Simon, Erez Berg, S. A. Parameswaran

2024Physical review. B./Physical review. B22 citationsDOIOpen Access PDF

Abstract

Magic-angle twisted bilayer graphene has attracted significant attention for its strongly correlated phenomena. Recent scanning tunneling experiments have measured graphene-scale Kekul\'e charge ordering in some of the correlated insulators and nearby metallic phases. While most of these can be explained by the strain-induced incommensurate Kekul\'e spiral phase, the presence of Kekul\'e ordering in ultralow strain devices is unexpected within the existing theory. Using Hartree-Fock and strong-coupling calculations, the authors show that such observations can be rationalized by invoking electron-phonon coupling to zone-corner graphene phonons.

Topics & Concepts

Bilayer grapheneGrapheneCoupling (piping)PhononCondensed matter physicsElectronPhysicsBilayerMaterials scienceQuantum mechanicsChemistryMembraneComposite materialBiochemistryGraphene research and applicationsQuantum and electron transport phenomenaFullerene Chemistry and Applications