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Study of anisotropy in the superconducting properties of FeTe<sub>0.55</sub>Se<sub>0.45</sub> single crystal grown by the self-flux method

Himanshu Chauhan, Rohit Kumar, G. D. Varma

2022Superconductor Science and Technology15 citationsDOI

Abstract

Abstract We report anisotropy in the superconducting properties of FeTe 0.55 Se 0.45 bulk single crystal synthesized via the self-flux method. We have performed magnetotransport, magnetic and heat capacity measurements on single crystals of same batch. The grown crystals have also been characterized by XRD, XPS and Raman measurements. The superconductivity at T C ∼ 14 K has been affirmed by the temperature-dependent resistivity, magnetic, and specific heat measurements. The anisotropy in the upper critical field ( H C2 ), coherence length ( ξ ), and critical current density ( J C ) have been studied from the magnetotransport and magnetic measurements, respectively, under applied magnetic fields of 0–12 T along the ab -plane and c -axis. The critical current density has been estimated by Bean’s critical state model at different magnetic fields ( J C ( H )) and temperatures ( J C ( T )) measured for H ‖ab-plane and H ‖ c axis. The anisotropic behaviour has also been observed for J C ( H ). The presence of ‘peak effect’ or fishtail characteristic has been noticed in M – H loops for H ‖ c only, which shows a shift towards the lower fields with increasing temperature. The nature of the pinning mechanisms in the sample has been determined by the normalized pinning force density using the Dew Hughes scaling rule, and the analysis of experimental data indicates the presence of δ l- pinning in the sample. The temperature-dependent electronic specific heat has been fitted with the exponential law and the evaluated coupling constant 2Δ 0 / k B T c is ∼3.42 which is close to the universal BCS value of 3.53. The observed low value of residual Sommerfeld coefficient <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mi>γ</mml:mi> <mml:mrow> <mml:mi>r</mml:mi> <mml:mi>e</mml:mi> <mml:mi>s</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> ≈ 4.59 mJ mol −1 K 2 indicates good quality of the grown single crystal.

Topics & Concepts

Condensed matter physicsSuperconductivityAnisotropyMaterials scienceElectrical resistivity and conductivitySingle crystalMagnetic fieldFlux pinningCoherence lengthHeat capacityCrystal (programming language)Raman spectroscopyCritical fieldNuclear magnetic resonanceHigh-temperature superconductivityPhysicsThermodynamicsOpticsProgramming languageComputer scienceQuantum mechanicsIron-based superconductors researchRare-earth and actinide compoundsPhysics of Superconductivity and Magnetism
Study of anisotropy in the superconducting properties of FeTe<sub>0.55</sub>Se<sub>0.45</sub> single crystal grown by the self-flux method | Litcius