Ultrastable electrolyte (>3500 hours at high current density) achieved by high-entropy solvation toward practical aqueous zinc metal batteries
Bin Xie, Chaohe Zheng, Haoran Lang, Min Li, Qiang Hu, Xin Tan, Qiaoji Zheng, Yu Huo, Jingxin Zhao, Jialin Yang, Zhen‐Yi Gu, Dunmin Lin, Xing‐Long Wu
Abstract
Ultrastable (>3500 h) electrolyte at high current density by high-entropy solvation for AZIBs. With increasing solvation configuration entropy, O–H bond order in active H 2 O and ionic conductivity are increased, realizing highly reversible Zn anode.
Topics & Concepts
SolvationElectrolyteAnodeAqueous solutionConductivityCurrent densityIonic conductivityEntropy (arrow of time)Ionic bondingInorganic chemistryZincMetalChemistryMaterials scienceThermodynamicsChemical physicsPhysical chemistryIonElectrodePhysicsMetallurgyOrganic chemistryQuantum mechanicsAdvanced battery technologies researchElectrocatalysts for Energy ConversionAdvanced Battery Materials and Technologies