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Maximum Chirality Empowered by a Bound State in a Continuum in a Plasmonic Metasurface

Hanan Ali, Simone Zanotti, Giovanni Pellegrini, Emilija Petronijevic, Lucio Claudio Andreani

2024ACS Applied Optical Materials19 citationsDOIOpen Access PDF

Abstract

Achieving a strong and robust chiral response in plasmonic metasurfaces is among the key goals of current nanophotonic research. In this work, we theoretically show that the circular dichroism (CD) of a metal metasurface can be maximized by exploiting the concept of a bound state in a continuum (BIC) with symmetry breaking. We consider a gold metasurface with a deformation of circular holes into oval holes. The chiral response at small values of the angle of incidence is dominated by a quasi-BIC, with nearly maximal values of the absorption CD that are almost independent of the deformation. A strong CD in emission is also demonstrated. Symmetry analysis and mode profiles show that the extrinsically chiral response does indeed follow from a symmetry-broken BIC and is associated with a strong enhancement of the local electrical field. The concept of a plasmonic BIC with symmetry breaking provides a robust pathway to increase the chiral response in metal metasurfaces and opens research opportunities in chiral plasmonics that combine narrow resonances with local field enhancement.

Topics & Concepts

PlasmonCircular dichroismChirality (physics)PhysicsMetamaterialSymmetry breakingSymmetry (geometry)NanophotonicsBound stateCondensed matter physicsOpticsQuantum mechanicsSpontaneous symmetry breakingGeometryCrystallographyChemistryExplicit symmetry breakingMathematicsMetamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon ResearchOrbital Angular Momentum in Optics
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