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Decarboxylative Hydroxylation of Benzoic Acids

Wanqi Su, Peng Xu, Tobias Ritter

2021Angewandte Chemie14 citationsDOIOpen Access PDF

Abstract

Abstract Herein, we report the first decarboxylative hydroxylation to synthesize phenols from benzoic acids at 35 °C via photoinduced ligand‐to‐metal charge transfer (LMCT)‐enabled radical decarboxylative carbometalation. The aromatic decarboxylative hydroxylation is synthetically promising due to its mild conditions, broad substrate scope, and late‐stage applications.

Topics & Concepts

HydroxylationChemistryPhenolsDecarboxylationSubstrate (aquarium)Organic chemistryBenzoic acidLigand (biochemistry)Combinatorial chemistryCatalysisReceptorEnzymeBiochemistryOceanographyGeologyRadical Photochemical ReactionsCatalytic C–H Functionalization MethodsSulfur-Based Synthesis Techniques