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Optical-Switch-Enabled Microfluidics for Sensitive Multichannel Colorimetric Analysis

Jiukai Tang, Xiaobao Cao, Guangyu Qiu, Andrew J. deMello, Jing Wang

2021Analytical Chemistry19 citationsDOIOpen Access PDF

Abstract

hip (OSEMC) fabricated by two-photon stereolithography. The integration of optical switches enables sequential signal readout from each detection channel, and thus, only a single light source and a photodetector are required for operation. Optical switches can be controlled in a bespoke manner by changing the medium in the switch channel between a "light-transmitting" fluid and a "light-blocking" fluid using pneumatic microvalves. Such optical switches are characterized by fast response times (approximately 200 ms), tunable switching frequencies (between 0.1 and 1.0 Hz studied), and excellent stability. Operational performance demonstrates both good sensitivity and reproducibility through the colorimetric analysis of nitrite and ammonium samples using four detection channels. Furthermore, the use of OSEMC for parallel and real-time analysis of flowing samples is investigated via characterization of the adsorption kinetics of tartrazine on activated charcoal and the catalytic reaction kinetics of horseradish peroxidase (HRP).

Topics & Concepts

MicrofluidicsChemistryMiniaturizationOptoelectronicsDetectorChannel (broadcasting)Optical switchPhotodiodePhotodetectorReproducibilitySensitivity (control systems)NanotechnologyOpticsElectronic engineeringMaterials scienceComputer scienceChromatographyTelecommunicationsEngineeringPhysicsMicrofluidic and Capillary Electrophoresis ApplicationsBiosensors and Analytical DetectionAdvanced Chemical Sensor Technologies
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