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<i>Ortho</i>-Selective amination of arene carboxylic acids <i>via</i> rearrangement of acyl <i>O</i>-hydroxylamines

James E. Gillespie, Nelson Y. S. Lam, Robert J. Phipps

2023Chemical Science15 citationsDOIOpen Access PDF

Abstract

Aromatic acyl O -hydroxylamines, synthesised in one straightforward step, undergo rearrangement under simple conditions to give ortho -aminated arenes. For benzoic acid-derived substrates, this leads directly to unprotected anthranilic acids.

Topics & Concepts

AminationChemistryCarboxylic acidCarroll rearrangementMedicinal chemistryOrganic chemistryStereochemistrySigmatropic reactionCatalysisSynthesis and Catalytic ReactionsCatalytic C–H Functionalization MethodsAsymmetric Hydrogenation and Catalysis
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