Breaking the scaling relationship of ORR on carbon-based single-atom catalysts through building a local collaborative structure
Cehuang Fu, Liuxuan Luo, Lijun Yang, Shuiyun Shen, Guanghua Wei, Junliang Zhang
Abstract
The local collaborative structure further stabilizes the OOH*/OH* and weakens the on metal site by hydrogen bond and repulsive interaction, for which the scaling relationship of ORR could be broken.
Topics & Concepts
CatalysisScalingAtom (system on chip)Hydrogen atomCarbon fibersMetalLocal structureCarbon atomHydrogen bondChemistryChemical physicsNanotechnologyMaterials scienceCrystallographyMoleculeComputer scienceOrganic chemistryRing (chemistry)MathematicsGeometryComposite numberAlkylEmbedded systemComposite materialElectrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceAmmonia Synthesis and Nitrogen Reduction