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Direct measurements for the fine-structure splitting of S viii and Cl ix

Qifeng Lu, C. L. Yan, G. Xu, Ning Fu, Y. Yang, Y. Zou, A. V. Volotka, Jun Xiao, Nobuyuki Nakamura, R. Hutton

2020Physical review. A/Physical review, A16 citationsDOI

Abstract

Using electron-beam ion traps (EBITs), we have made direct measurements for the fine-structure splitting $2{p}^{5}$ of S viii and Cl ix, which are important to the test of ab initio theory in F-like ions. Their wavelength are redetermined in the laboratory with an accuracy of 23 ppm, i.e., $10\phantom{\rule{4pt}{0ex}}085.40\ifmmode\pm\else\textpm\fi{}0.23\phantom{\rule{4pt}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1}$ for S viii, where the early value observed in the solar spectrum is questionable, and $13\phantom{\rule{4pt}{0ex}}643.39\ifmmode\pm\else\textpm\fi{}0.32\phantom{\rule{4pt}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1}$ for Cl ix, where only indirect measurements had been performed. High-precision calculations, including ab initio treatment of QED effects, are accomplished for $10\ensuremath{\le}Z\ensuremath{\le}18$ and compared with the experimental results. Good agreement is found between our experimental and theoretical values of the fine-structure energy among these ions except for Al v, which calls for further investigations. Besides, we have succeeded in pushing EBIT operation towards the infrared spectral region relevant to astrophysics.

Topics & Concepts

PhysicsFine structureAb initioIonAtomic physicsAb initio quantum chemistry methodsEnergy (signal processing)WavelengthCondensed matter physicsOpticsQuantum mechanicsMoleculeExcitonAtomic and Molecular PhysicsLaser-induced spectroscopy and plasmaMass Spectrometry Techniques and Applications
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