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Fermi Surface Nesting Driving the RKKY Interaction in the Centrosymmetric Skyrmion Magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>Gd</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi>PdSi</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>

Yuyang Dong, Yosuke Arai, Kenta Kuroda, Masayuki Ochi, Natsumi Tanaka, Yuxuan Wan, Matthew D. Watson, T. K. Kim, Céphise Cacho, Makoto Hashimoto, Dong-Hui Lu, Yuji Aoki, Tatsuma D. Matsuda, Takeshi Kondo

2024Physical Review Letters12 citationsDOIOpen Access PDF

Abstract

The magnetic skyrmions generated in a centrosymmetric crystal were recently first discovered in Gd_{2}PdSi_{3}. In light of this, we observe the electronic structure by angle-resolved photoemission spectroscopy and unveil its direct relationship with the magnetism in this compound. The Fermi surface and band dispersions are demonstrated to have a good agreement with the density functional theory calculations carried out with careful consideration of the crystal superstructure. Most importantly, we find that the three-dimensional Fermi surface has extended nesting which matches well the q vector of the magnetic order detected by recent scattering measurements. The consistency we find among angle-resolved photoemission spectroscopy, density functional theory, and the scattering measurements suggests the Ruderman-Kittel-Kasuya-Yosida interaction involving itinerant electrons to be the formation mechanism of skyrmions in Gd_{2}PdSi_{3}.

Topics & Concepts

Fermi surfaceSkyrmionPhotoemission spectroscopyCondensed matter physicsPhysicsAngle-resolved photoemission spectroscopyDensity functional theoryFermi levelMagnetismScatteringSuperstructureElectronic structureElectronQuantum mechanicsSpectral lineThermodynamicsSuperconductivityMagnetic properties of thin filmsMagnetic and transport properties of perovskites and related materialsPhysics of Superconductivity and Magnetism
Fermi Surface Nesting Driving the RKKY Interaction in the Centrosymmetric Skyrmion Magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>Gd</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi>PdSi</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> | Litcius