Litcius/Paper detail

Thermokinetic model establishment and numerical simulation of 2,4,6-trinitrophenol based on eco-friendly synthesis method

Ye-Cheng Liu, An‐Chi Huang, Yan Tang, Xiaoming Ma, Ya-Ping Yang, Zhihao Wu, Chi‐Min Shu, Zhixiang Xing, Juncheng Jiang

2021Journal of Energetic Materials11 citationsDOI

Abstract

In this paper, the synthesis of 2,4,6-trinitrophenol from phenol was improved in the range of 0–65°C, and the yield was 79.4%. The effectiveness of the synthesis process was confirmed by Nuclear Magnetic Resonance, Fourier Transform Infrared Spectrometer, and Scanning Electron Microscope. The thermal stability of the product was further studied by differential scanning calorimetry and accelerating rate calorimeter. The kinetic model established by combining linear regression and nonlinear regression methods shows that the apparent activation energy of the energetic material synthesized under the green process is about 130 kJ/mol.

Topics & Concepts

Differential scanning calorimetryYield (engineering)PhenolFourier transform infrared spectroscopyScanning electron microscopeKinetic energyFourier transformThermal stabilityActivation energyAnalytical Chemistry (journal)ChemistryThermal analysisMaterials scienceThermalThermodynamicsChemical engineeringPhysical chemistryPhysicsOrganic chemistryComposite materialMathematicsEngineeringMathematical analysisQuantum mechanicsEnergetic Materials and CombustionThermal and Kinetic AnalysisChemistry and Chemical Engineering