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Hyperbolic enhancement of photocurrent patterns in minimally twisted bilayer graphene

S. S. Sunku, D. Halbertal, T. Stauber, S. Chen, A. S. McLeod, A. Rikhter, M. E. Berkowitz, C. F. B. Lo, D. E. Gonzalez-Acevedo, J. C. Hone, C. R. Dean, M. M. Fogler, D. N. Basov

2021Nature Communications56 citationsDOIOpen Access PDF

Abstract

Quasi-periodic moiré patterns and their effect on electronic properties of twisted bilayer graphene have been intensely studied. At small twist angle θ, due to atomic reconstruction, the moiré superlattice morphs into a network of narrow domain walls separating micron-scale AB and BA stacking regions. We use scanning probe photocurrent imaging to resolve nanoscale variations of the Seebeck coefficient occurring at these domain walls. The observed features become enhanced in a range of mid-infrared frequencies where the hexagonal boron nitride substrate is optically hyperbolic. Our results illustrate the capabilities of the nano-photocurrent technique for probing nanoscale electronic inhomogeneities in two-dimensional materials.

Topics & Concepts

PhotocurrentMaterials scienceSuperlatticeNanoscopic scaleStackingSubstrate (aquarium)Bilayer grapheneBilayerCondensed matter physicsGrapheneOptoelectronicsSeebeck coefficientPhotoconductivityRange (aeronautics)Thermoelectric effectNanostructureNanotechnologyHexagonal boron nitrideDomain wall (magnetism)Graphene nanoribbonsScalingMicrocrystallineTwistDomain (mathematical analysis)Characterization (materials science)HeterojunctionHexagonal crystal systemAtomic unitsGraphene research and applications2D Materials and ApplicationsTopological Materials and Phenomena
Hyperbolic enhancement of photocurrent patterns in minimally twisted bilayer graphene | Litcius