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Configurational control of low-symmetry heteroleptic metal–organic cages with asymmetric ligands

Hao Yu, Ziteng Guo, Jie Tang, Ningxu Han, Junjuan Shi, Meng Li, Houyu Zhang, Ming Wang

2025Chemical Science11 citationsDOIOpen Access PDF

Abstract

to undergo a structural transformation and selectively assemble into a single dominant configuration from 13 potential isomers. This work not only demonstrates the immense potential of integrating asymmetric ligand assembly with multi-ligand co-assembly strategies but also highlights the critical role of steric effects in guiding assembly pathways and achieving precise configurational control in low-symmetry MOCs.

Topics & Concepts

Symmetry (geometry)MetalControl (management)ChemistryComputational chemistryCombinatorial chemistryMaterials scienceOrganic chemistryMathematicsComputer scienceGeometryArtificial intelligenceSupramolecular Chemistry and ComplexesMagnetism in coordination complexesCrystallography and molecular interactions