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Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi <sub>2</sub> Sr <sub>2</sub> LaCuO <sub>6+δ</sub>

Jiemin Li, Abhishek Nag, Jonathan Pelliciari, H. C. Robarts, A. C. Walters, Mirian García‐Fernández, Hiroshi Eisaki, Dongjoon Song, Hong Ding, Steven Johnston, Riccardo Comin, Ke‐Jin Zhou

2020Proceedings of the National Academy of Sciences53 citationsDOIOpen Access PDF

Abstract

Significance Charge-density waves (CDWs) are a ubiquitous form of electron density modulation in cuprate superconductors. Unveiling the nature of quasistatic CDWs and their dynamical excitations is crucial for understanding their origin––similar to the study of antiferromagnetism in cuprates. However, dynamical CDW excitations remain largely unexplored due to the limited availability of suitable experimental probes. Here, using resonant inelastic X-ray scattering, we observe dynamical CDW excitations in Bi 2 Sr 2 LaCuO 6+δ (Bi2201) superconductors through its interference with the lattice. The distinct anomalies of the bond-buckling and the bond-stretching phonons allow us to draw a clear picture of funnel-shaped dynamical CDW excitations in Bi2201. Our results of the interplay between CDWs and the phonon anomalies shed light on the nature of CDWs in cuprates.

Topics & Concepts

Condensed matter physicsCupratePhononSuperconductivityPhysicsCharge density waveAtomic orbitalCharge densityValence (chemistry)ElectronQuantum mechanicsPhysics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsMagnetic and transport properties of perovskites and related materials