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Multi-Particle Three-Dimensional Covariance Imaging: “Coincidence” Insights into the Many-Body Fragmentation of Strong-Field Ionized D<sub>2</sub>O

Felix Allum, Chuan Cheng, Andrew J. Howard, P. H. Bucksbaum, M. Brouard, Thomas Weinacht, Ruaridh Forbes

2021The Journal of Physical Chemistry Letters29 citationsDOIOpen Access PDF

Abstract

dissociation on the intensity of the ionizing laser, revealing mechanistic insights into the nuclear dynamics driven during the laser pulse. The experimental methodology laid out, with its drastic reduction in acquisition time, is expected to be of great benefit to future photofragment imaging studies.

Topics & Concepts

CovarianceCoincidenceIonizationPhysicsFragmentation (computing)Covariance mappingDissociation (chemistry)Computational physicsDetectorAtomic physicsCovariance functionChemistryIonOpticsStatisticsMathematicsComputer scienceQuantum mechanicsMedicineCovariance intersectionPathologyAlternative medicinePhysical chemistryOperating systemLaser-Matter Interactions and ApplicationsMass Spectrometry Techniques and ApplicationsAdvanced Chemical Physics Studies
Multi-Particle Three-Dimensional Covariance Imaging: “Coincidence” Insights into the Many-Body Fragmentation of Strong-Field Ionized D<sub>2</sub>O | Litcius