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Isolable Pyridinium Trifluoromethoxide Salt for Nucleophilic Trifluoromethoxylation

Geraldo Duran-Camacho, Devin M. Ferguson, Jeff W. Kampf, Douglas C. Bland, Melanie S. Sanford

2021Organic Letters37 citationsDOI

Abstract

An isolable pyridinium trifluoromethoxide salt is prepared from the reaction of 4-dimethylaminopyridine with the commercially available liquid 2,4-dinitro(trifluoromethoxy)benzene. The salt is an effective trifluoromethoxide source for SN2 reactions to form trifluoromethyl ethers.

Topics & Concepts

ChemistryPyridiniumSalt (chemistry)SN2 reactionNucleophileBenzeneTrifluoromethylOrganic chemistryMedicinal chemistryCatalysisAlkylFluorine in Organic ChemistrySynthesis and Reactions of Organic CompoundsSynthesis and Biological Evaluation
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