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Selective Electrochemical Oxidation of Functionalized Pyrrolidines

Nicholas R. Deprez, Dane J. Clausen, Jia‐Xuan Yan, Feng Peng, Shaoguang Zhang, Jongrock Kong, Yanguang Bai

2021Organic Letters24 citationsDOI

Abstract

A method for the selective electrochemical aminoxyl-mediated Shono-type oxidation of pyrrolidines to pyrrolidinones is described. These transformations show the high selectivity and functional group compatibility. This chemistry also demonstrates the use of an operationally simple ElectraSyn 2.0 and cost-effective stainless-steel electrode for the electrochemical oxidation of functionalized pyrrolidines.

Topics & Concepts

ChemistryElectrochemistryCombinatorial chemistryCompatibility (geochemistry)SelectivityPyrrolidinonesElectrodeFunctional groupOrganic chemistryPolymerChemical engineeringCatalysisPhysical chemistryEngineeringOxidative Organic Chemistry ReactionsRadical Photochemical ReactionsAdvanced Synthetic Organic Chemistry
Selective Electrochemical Oxidation of Functionalized Pyrrolidines | Litcius