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Electrical and optical properties of transition metal dichalcogenides on talc dielectrics

Darren Nutting, Gabriela Augusta Prando, Marion E. Severijnen, Ingrid D. Barcelos, Shi Guo, Peter C. M. Christianen, U. Zeitler, Y. Galvão Gobato, Freddie Withers

2021Nanoscale36 citationsDOIOpen Access PDF

Abstract

Advanced van der Waals (vdW) heterostructure devices rely on the incorporation of high quality dielectric materials which need to possess a low defect density as well as being atomically smooth and uniform. In this work we explore the use of talc dielectrics as a potentially clean alternative substrate to hexagonal boron nitride (hBN) for few-layer transition metal dichalcogenide (TMDC) transistors and excitonic TMDC monolayers. We find that talc dielectric transistors show small hysteresis which does not depend strongly on sweep rate and show negligible leakage current for our studied dielectric thicknesses. We also show narrow photoluminescence linewidths down to 10 meV for different TMDC monolayers on talc which highlights that talc is a promising material for future van der Waals devices.

Topics & Concepts

TalcDielectricMaterials sciencevan der Waals forceTransition metalMetalOptoelectronicsNanotechnologyComposite materialMetallurgyChemistryMoleculeBiochemistryOrganic chemistryCatalysis2D Materials and ApplicationsGraphene research and applicationsLuminescence and Fluorescent Materials
Electrical and optical properties of transition metal dichalcogenides on talc dielectrics | Litcius