Litcius/Paper detail

Evolution of the Ferroelectric Properties of AlScN Film by Electrical Cycling with an Inhomogeneous Field Distribution

Kyung Do Kim, Yong Bin Lee, Suk Hyun Lee, In Soo Lee, Seung Kyu Ryoo, Seungyong Byun, Jae Hoon Lee, Hani Kim, Hyeon Woo Park, Cheol Seong Hwang

2023Advanced Electronic Materials56 citationsDOIOpen Access PDF

Abstract

Abstract This work investigates the evolution of the ferroelectric (FE) performance of the sputtered aluminum scandium nitride (AlScN) thin film, which has a high remanent polarization ( P r , > 100 µC cm −2 ) and coercive field ( E c , > 6 MV cm −1 ), with the electric field cycling. The work aims at elucidating the underlying origin of the severe fatigue behavior, even with a relatively small number of endurance cycles (<10 5 ). When cycled with a low electric field, an internal field is created by charges trapped between the FE layer and the interfacial dielectric layer (non‐FE). On the other hand, fatigue is observed when cycled with a high electric field cycling. This work proposes a new method to simulate a switching current utilizing an inhomogeneous field mechanism and the appropriate circuit model to assess the thickness change of the non‐FE layer. It is concluded that the thickened non‐FE layer after the field cycling results in fatigue.

Topics & Concepts

Materials scienceCyclingElectric fieldFerroelectricityCoercivityPolarization (electrochemistry)DielectricScandiumComposite materialField (mathematics)ElectrodeLayer (electronics)AluminiumNitrideWork functionCondensed matter physicsOptoelectronicsMetallurgyPure mathematicsHistoryMathematicsChemistryArchaeologyPhysical chemistryQuantum mechanicsPhysicsAcoustic Wave Resonator TechnologiesFerroelectric and Negative Capacitance DevicesFerroelectric and Piezoelectric Materials