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Multi-Synergistic Removal of Low-Boiling-Point Contaminants with Efficient Carbon Aerogel-Based Solar Purifier

Zhongming Huang, Yingpeng Wan, Jianli Liang, Yafang Xiao, Xiaozhen Li, Xiao Cui, Shuang Tian, Qi Zhao, Shengliang Li, Chun‐Sing Lee

2021ACS Applied Materials & Interfaces32 citationsDOI

Abstract

Solar steam generation is considered as an efficient way for addressing water shortage issues via seawater desalination and wastewater purification. In a solar evaporator, an absorber would convert optical energy to heat for evaporating nearby water. In this process, many low-boiling-point contaminants can also be evaporated along with water steam, which compromises the effectiveness of purification. There is, so far, no study on the removal of such low-boiling-point contaminants such as organic pesticides in wastewater. To address this problem, we demonstrate a versatile carbon hybrid aerogel (CHA) as a solar powered water purification platform. With an elaborate absorber design, the maximum solar evaporation rate of 2.1 kg m–2 h–1 is achieved under 1 sun illumination. More importantly, CHA can effectively suppress the evaporation of low-boiling-point contaminants including common pesticides and mercury ion via its strong adsorption and retention effect. Synergetic steaming and the adsorption of CHA will inspire more paradigms of solar steam generation technologies for applications relevant to detoxification and water remediation.

Topics & Concepts

Boiling pointDesalinationMaterials sciencePortable water purificationSolar energyBoilingAerogelAdsorptionEvaporatorEnvironmental remediationEvaporationWastewaterGroundwater remediationWater treatmentWaste managementContaminationEnvironmental scienceHeat exchangerChemical engineeringEnvironmental engineeringNanotechnologyChemistryEngineeringOrganic chemistryBiochemistryEcologyThermodynamicsPhysicsBiologyMembraneSolar-Powered Water Purification MethodsMembrane Separation TechnologiesSurface Modification and Superhydrophobicity
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