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Near-Unity Light–Matter Interaction in Mid-Infrared van der Waals Metasurfaces

Haonan Ling, Milad Nourbakhsh, Vincent R. Whiteside, Joseph G. Tischler, Artur R. Davoyan

2024Nano Letters14 citationsDOI

Abstract

Accessing mid-infrared radiation is of great importance for a range of applications, including thermal imaging, sensing, and radiative cooling. Here, we study light interaction with hexagonal boron nitride (hBN) nanocavities and reveal strong and tunable resonances across its hyperbolic transition. In addition to conventional phonon-polariton excitations, we demonstrate that the high refractive index of hexagonal boron nitride outside the Reststrahlen band allows enhanced light–matter interactions in deep subwavelength (<λ/15) nanostructures across a broad 7–8 μm range. Emergence and interplay of Fabry–Perot and Mie-like resonances are examined experimentally and theoretically. Near-unity absorption and high quality ( Q ≥ 80) resonance interaction in the vicinity of the hBN transverse optical phonon is further observed. Our study provides avenues to design highly efficient and ultracompact structures for controlling mid-infrared radiation and accessing strong light–matter interactions with hBN.

Topics & Concepts

van der Waals forcePolaritonInfraredMaterials sciencePhononResonance (particle physics)OptoelectronicsRefractive indexAbsorption (acoustics)Condensed matter physicsMolecular physicsPhysicsOpticsAtomic physicsMoleculeQuantum mechanicsThermal Radiation and Cooling TechnologiesMetamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon Research