Litcius/Paper detail

Low-Temperature Direct Growth of Amorphous Boron Nitride Films for High-Performance Nanoelectronic Device Applications

Seyed Mehdi Sattari‐Esfahlan, Hyoung Gyun Kim, Sang Hwa Hyun, Jun‐Hui Choi, Hyun Sik Hwang, Eui‐Tae Kim, Hyeongsik Park, Jae‐Hyun Lee

2023ACS Applied Materials & Interfaces35 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide We successfully demonstrated the improvement and stabilization of the electrical properties of a graphene field effect transistor by fabricating a sandwiched amorphous boron nitride (a-BN)/graphene (Gr)/a-BN using a directly grown a-BN film. The a-BN film was grown via low-pressure chemical vapor deposition (LPCVD) at a low growth temperature of 250 °C and applied as a protection layer in the sandwiched structure. Both structural and chemical states of the as-grown a-BN were verified by various spectroscopic and microscopic analyses. We analyzed the Raman spectra of Gr/SiO 2 and a-BN/Gr/a-BN structures to determine the stability of the device under exposure to ambient air. Following exposure, the intensity of the 2D/G-peak ratio of Gr/SiO 2 decreased and the position of the G and 2D peaks red-shifted due to the degradation of graphene. In contrast, the peak position of encapsulated graphene is almost unchanged. We also confirmed that the mobility of a-BN/Gr/a-BN structure is 17,941 cm 2 /Vs. This synthetic strategy could provide a facile way to synthesize uniform a-BN film for encapsulating various van der Waals materials, which is beneficial for future applications in nanoelectronics.

Topics & Concepts

Materials scienceGrapheneRaman spectroscopyChemical vapor depositionBoron nitrideAmorphous solidNanotechnologyBoronChemical engineeringElectron mobilityOptoelectronicsCrystallographyOpticsOrganic chemistryPhysicsChemistryEngineeringGraphene research and applications2D Materials and ApplicationsDiamond and Carbon-based Materials Research