Litcius/Paper detail

Covalent organic framework‐supported Pd nanoparticles: An efficient and reusable heterogeneous catalyst for Suzuki–Miyaura coupling reactions

Hao Jin, Chi Zhang, Pingwei Liu, Xin Ge, Shaodong Zhou

2022Applied Organometallic Chemistry26 citationsDOI

Abstract

Abstract A Schiff base hollow covalent organic framework (COF) was used for anchoring Pd(II) to synthesize the Pd@COF‐TB nanocatalyst. Then, the as‐synthesized Pd@COF‐TB catalyst has been meticulously characterized using several methods. Thereafter, the catalytic performance of the Pd@COF‐TB species regarding Suzuki–Miyaura coupling reactions was examined, and the corresponding products were obtained with good to excellent yields. Besides, the Pd@COF‐TB catalyst could be recovered conveniently and reused at least eight times without obvious decrease in activity and selectivity. More importantly, the leaching of Pd during the reaction process could be negligible, which is crucially important when preparing bioactive species.

Topics & Concepts

Covalent organic frameworkChemistryCatalysisCovalent bondSchiff baseSelectivityLeaching (pedology)NanoparticleCoupling reactionPalladiumCombinatorial chemistryOrganic chemistryPolymer chemistryChemical engineeringSoil scienceEnvironmental scienceSoil waterEngineeringCovalent Organic Framework ApplicationsMetal-Organic Frameworks: Synthesis and ApplicationsCatalytic Cross-Coupling Reactions