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Bipolar HiPIMS: The role of capacitive coupling in achieving ion bombardment during growth of dielectric thin films

Hao Du, Michal Zanáška, N. Brenning, Ulf Helmersson

2021Surface and Coatings Technology27 citationsDOIOpen Access PDF

Abstract

Bipolar high-power impulse magnetron sputtering (HiPIMS) is used to achieve ion acceleration for ion bombardment of dielectric thin films . This is realized by increasing the plasma potential ( U p ), during the interval in-between the HiPIMS-pulses, using a positive reversed voltage ( U rev ). As long as the film surface potential ( U s ) is maintained low, close to ground potential, this increase in U p results in ion-acceleration as ions approach the film surface. The effect of U rev on the ion bombardment is demonstrated by the growth of dielectric (Al,Cr) 2 O 3 films on two sets of substrates, Si (001) and sapphire (0001) utilizing a U rev ranging from 0 to 300 V. A clear ion bombardment effect is detected in films grown on the conductive Si substrate, while no, or a very small, effect is observed in films grown on the dielectric sapphire substrate . This is ascribed to the changes in U s when the substrate is subjected to the bombardment of positive ions . For a film surface that has a high capacitance to ground, U s remains close to ground potential for an extended time in-between the HiPIMS pulses, while if the capacitance is low, U s quickly attains floating potential ( U float ) close to U p . The simulated temporal evolutions of U s for the films by using capacitors show that for a 1 μm thick (Al,Cr) 2 O 3 film on a conductive substrate, U s is maintained close to ground potential during the entire 20 μs that U rev is applied after the HiPIMS pulse. On the other hand, when a capacitance corresponding to the 0.5 mm thick sapphire substrate is used, U s rapidly attains a potential close to U rev .

Topics & Concepts

High-power impulse magnetron sputteringMaterials scienceDielectricIonSubstrate (aquarium)Thin filmOptoelectronicsAcceleration voltageSapphireCapacitanceSputter depositionSputteringAnalytical Chemistry (journal)OpticsNanotechnologyChemistryLaserPhysicsElectrodeElectronCathode rayOceanographyChromatographyOrganic chemistryGeologyQuantum mechanicsPhysical chemistryMetal and Thin Film MechanicsSemiconductor materials and devicesPlasma Diagnostics and Applications