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Eco-techno-economic analysis of onboard membrane carbon capture and storage systems considering CO2/N2 and CO2/O2 selectivity improvements

Hongkyoung Shin, Abduljelil Worku Sabir, Juyoung Oh, Pyung Soo Lee, Youngsub Lim

2025Separation and Purification Technology8 citationsDOIOpen Access PDF

Abstract

The shipping industry aims to achieve net zero emissions, and compact-sized membrane-based onboard carbon capture and storage systems can be a feasible solution. However, most previous studies have overlooked the importance of CO 2 /O 2 separation performance, leading to higher energy consumption and operating expenditures. In this study, a three-stage membrane carbon capture system was integrated with a precooled Linde–Hampson liquefaction process to minimize CO 2 avoidance costs while adhering to the FuelEU Maritime regulations. Two case studies assessed the impact of CO 2 /N 2 and CO 2 /O 2 selectivity improvements: one with a fixed greenhouse gas intensity target (62.90 g CO2eq /MJ, 2040–44 target) and another with varying targets. The results show that enhancing selectivity for not only CO 2 /N 2 but also CO 2 /O 2 is essential for developing cost-effective and energy-efficient onboard membrane carbon capture and storage systems, making it a feasible solution.

Topics & Concepts

Carbon capture and storage (timeline)Carbon fibersSelectivityEnvironmental scienceCarbon dioxideProcess engineeringCo2 removalWaste managementChemical engineeringChemistryMaterials scienceEngineeringClimate changeCatalysisOrganic chemistryGeologyComposite numberComposite materialOceanographyMembrane Separation and Gas TransportMembrane Separation TechnologiesMembrane-based Ion Separation Techniques