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Attosecond optoelectronic field measurement in solids

Shawn Sederberg, Dmitry A. Zimin, Sabine Keiber, Florian Siegrist, Michael S. Wismer, Vladislav S. Yakovlev, Isabella Floss, C. Lemell, Joachim Burgdörfer, Martin Schultze, Ferenc Krausz, Nicholas Karpowicz

2020Nature Communications138 citationsDOIOpen Access PDF

Abstract

The sub-cycle interaction of light and matter is one of the key frontiers of inquiry made accessible by attosecond science. Here, we show that when light excites a pair of charge carriers inside of a solid, the transition probability is strongly localized to instants slightly after the extrema of the electric field. The extreme temporal localization is utilized in a simple electronic circuit to record the waveforms of infrared to ultraviolet light fields. This form of petahertz-bandwidth field metrology gives access to both the modulated transition probability and its temporal offset from the laser field, providing sub-fs temporal precision in reconstructing the sub-cycle electronic response of a solid state structure.

Topics & Concepts

AttosecondExtreme ultravioletMetrologyOffset (computer science)LaserPhysicsElectric fieldLight fieldOptoelectronicsField (mathematics)Maxima and minimaOpticsComputer scienceUltrashort pulseQuantum mechanicsPure mathematicsMathematical analysisProgramming languageMathematicsLaser-Matter Interactions and ApplicationsTerahertz technology and applicationsSpectroscopy and Quantum Chemical Studies