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Quantifiable polarity match effect on C–H bond cleavage reactivity and its limits in reaction design

Mauricio Maldonado‐Domínguez, Martin Srnec

2023Dalton Transactions12 citationsDOIOpen Access PDF

Abstract

When oxidants favour cleaving a strong C–H bond at the expense of weaker ones, which are otherwise inherently preferred due to their favourable reaction energy, reactivity factors such as the polarity match effect are often invoked.

Topics & Concepts

ElectrophileReactivity (psychology)NucleophileChemistryPolarity (international relations)A priori and a posterioriBond cleavageComputational chemistryStereochemistryCatalysisOrganic chemistryEpistemologyAlternative medicineCellMedicinePhilosophyPathologyBiochemistryCatalytic C–H Functionalization MethodsSynthesis and Catalytic ReactionsSulfur-Based Synthesis Techniques
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