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Pre-regulation of the planar chirality of pillar[5]arenes for preparing discrete chiral nanotubes

Shixin Fa, Keisuke Adachi, Yuuya Nagata, Kouichi Egami, Kenichi Kato, Tomoki Ogoshi

2021Chemical Science40 citationsDOIOpen Access PDF

Abstract

pre-regulation of the building blocks' chirality, which is different from frequently used post-regulation strategies. The planar chirality of rim-differentiated pillar[5]arenes is initially regulated by chiral awakening and further induction/inversion through stepwise achiral external stimuli. The pre-regulated chiral information is well stored in discrete nanotubes by interacting with a per-alkylamino-substituted pillar[5]arene. Such pre-regulation is more efficient than post-regulating the chirality of nanotubes.

Topics & Concepts

PillarChirality (physics)PlanarPlanar chiralityNanotechnologyMaterials scienceChemistryEnantioselective synthesisCatalysisOrganic chemistryPhysicsComputer scienceEngineeringQuantum mechanicsChiral symmetryMechanical engineeringComputer graphics (images)Nambu–Jona-Lasinio modelQuarkSupramolecular Chemistry and ComplexesSynthesis and Properties of Aromatic CompoundsSupramolecular Self-Assembly in Materials
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