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Nickel-Catalyzed Electrochemical Cyclizative Carboxylation of Alkene-Tethered Carbamoyl Chlorides with Carbon Dioxide

Linlin Wang, Xiaofei Liu, Wen‐Zhen Zhang, He Wang, Tao Li, Jian Huang, Wei‐Min Ren, Xiao‐Bing Lu

2023Synthesis10 citationsDOI

Abstract

Abstract Nickel-catalyzed electrochemical cyclizative carboxylation of alkene-tethered carbamoyl chlorides with atmospheric carbon dioxide in an undivided cell under simple constant current conditions is reported. This reaction is conducted with high efficiency under mild conditions, providing a convenient and green access to valuable 2-oxoindolin-3-ylacetic acids and 2-oxo-tetrahydroquinoline-4-carboxylic acids.

Topics & Concepts

ChemistryCarboxylationAlkeneCatalysisNickelElectrochemistryCarbon dioxideOrganic chemistryInorganic chemistryCombinatorial chemistryElectrodePhysical chemistryCarbon dioxide utilization in catalysisCO2 Reduction Techniques and CatalystsCatalytic C–H Functionalization Methods
Nickel-Catalyzed Electrochemical Cyclizative Carboxylation of Alkene-Tethered Carbamoyl Chlorides with Carbon Dioxide | Litcius