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Elastic moduli fluctuations predict wave attenuation rates in glasses

Geert Kapteijns, David Richard, Eran Bouchbinder, Edan Lerner

2021The Journal of Chemical Physics44 citationsDOIOpen Access PDF

Abstract

The disorder-induced attenuation of elastic waves is central to the universal low-temperature properties of glasses. Recent literature offers conflicting views on both the scaling of the wave attenuation rate Γ(ω) in the low-frequency limit (ω → 0) and its dependence on glass history and properties. A theoretical framework—termed Fluctuating Elasticity Theory (FET)—predicts low-frequency Rayleigh scattering scaling in đ spatial dimensions, Γ(ω) ∼ γ ω đ+1, where γ = γ(Vc) quantifies the coarse-grained spatial fluctuations of elastic moduli, involving a correlation volume Vc that remains debated. Here, using extensive computer simulations, we show that Γ(ω) ∼ γω3 is asymptotically satisfied in two dimensions ( đ = 2) once γ is interpreted in terms of ensemble—rather than spatial—averages, where Vc is replaced by the system size. In doing so, we also establish that the finite-size ensemble-statistics of elastic moduli is anomalous and related to the universal ω4 density of states of soft quasilocalized modes. These results not only strongly support FET but also constitute a strict benchmark for the statistics produced by coarse-graining approaches to the spatial distribution of elastic moduli.

Topics & Concepts

AttenuationScalingElastic modulusPhysicsElasticity (physics)Statistical physicsModuliRayleigh scatteringSpatial correlationScatteringCondensed matter physicsStatisticsOpticsQuantum mechanicsMathematicsThermodynamicsGeometryMaterial Dynamics and PropertiesGlass properties and applicationsBuilding materials and conservation