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Facile <i>in situ</i> reductive synthesis of both nitrogen deficient and protonated g-C<sub>3</sub>N<sub>4</sub> nanosheets for the synergistic enhancement of visible-light H<sub>2</sub> evolution

Weisong Li, Zheng Guo, Litong Jiang, Lei Zhong, Guoning Li, Jiajun Zhang, Kai Fan, Sergio González-Cortés, Kuijuan Jin, Chunjian Xu, Tiancun Xiao, Peter P. Edwards

2020Chemical Science83 citationsDOIOpen Access PDF

Abstract

Nitrogen deficient and protonated g-C<sub>3</sub>N<sub>4</sub> was fabricated by the conjoint protocol utilizing NH<sub>4</sub>Cl as gas template and H<sub>3</sub>PO<sub>2</sub> as doping agent, leading to enhanced visible-light harvesting and charge carrier separation to achieve efficient H<sub>2</sub> evolution.

Topics & Concepts

ProtonationNitrogenDopingIn situVisible spectrumMaterials scienceNanotechnologyChemistryOptoelectronicsOrganic chemistryIonAdvanced Photocatalysis TechniquesNanocluster Synthesis and ApplicationsMXene and MAX Phase Materials
Facile <i>in situ</i> reductive synthesis of both nitrogen deficient and protonated g-C<sub>3</sub>N<sub>4</sub> nanosheets for the synergistic enhancement of visible-light H<sub>2</sub> evolution | Litcius