Litcius/Paper detail

<i>Pas de Deux</i> of an NO Couple: Synchronous Photoswitching from a Double‐Linear to a Double‐Bent Ru(NO)<sub>2</sub> Core under Nitrosyl Charge Conservation

Asma Hasil, Daniel Beck, Daniel Schröder, Sébastien Pillet, Emmanuel Wenger, Theo Woike, Peter Klüfers, Dominik Schaniel

2022Angewandte Chemie International Edition11 citationsDOIOpen Access PDF

Abstract

Abstract The {Ru(NO) 2 } 10 dinitrosylruthenium complex [Ru(NO) 2 (PPh 3 ) 2 ] ( 1 ) shows photo‐induced linkage isomerism (PLI) of a special kind: the two NO ligands switch, on photo‐excitation, synchronously from the ground state (GS) with two almost linear RuNO functions to a metastable state (MS) which persists up to 230 K and can be populated to ≈50 %. The MS was experimentally characterised by photo‐crystallography, IR spectroscopy and DS‐calorimetry as a double‐bent variant of the double‐linear GS. The experimental results are confirmed by computation which unravels the GS/MS transition as a disrotatory synchronous 50° turn of the two nitrosyl ligands. Although 1 shows the usual redshift of the N−O stretch on bending the MNO unit, there is no increased charge transfer from Ru to NO along the GS‐to‐MS path. In terms of the effective‐oxidation‐state (EOS) method, both isomers of 1 and the transition state are Ru −II (NO + ) 2 species.

Topics & Concepts

ChemistryMetastabilityGround stateBent molecular geometryCrystallographyConrotatory and disrotatoryCharge (physics)PhysicsSpectroscopyState (computer science)FrustrationAtomic physicsStereochemistryCondensed matter physicsMathematicsQuantum mechanicsRing (chemistry)Organic chemistryAlgorithmPhotochromic and Fluorescence ChemistryPhotoreceptor and optogenetics researchRadical Photochemical Reactions