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The challenges in reliable determination of degradation rates and lifetime in polymer electrolyte membrane fuel cells

Qian Zhang, Corinna Harms, Jens Mitzel, Pawel Gazdzicki, K. Andreas Friedrich

2021Current Opinion in Electrochemistry31 citationsDOIOpen Access PDF

Abstract

The durability of polymer electrolyte membrane fuel cells (PEMFCs) needs to be further improved to cope with application requirements and economic competitiveness. This article highlights the challenges in the reliable determination of degradation rates and lifetime. The reliable evaluation of performance degradation rates is fundamental to quantify and benchmark durability and to allow comparisons between PEMFC durability tests performed using different materials or in different laboratories. The use of efficient recovery procedures enables the discrimination of reversible and irreversible voltage losses and facilitates the understanding of recovery mechanisms. In the end, recent contributions about lifetime diagnoses and prediction are presented, which are promising to be implemented in PEMFC applications.

Topics & Concepts

DurabilityElectrolyteDegradation (telecommunications)Benchmark (surveying)Proton exchange membrane fuel cellMaterials sciencePolymerFuel cellsMembraneComputer scienceVoltageProcess engineeringReliability engineeringChemical engineeringChemistryComposite materialEngineeringElectrical engineeringElectrodeTelecommunicationsBiochemistryPhysical chemistryGeodesyGeographyFuel Cells and Related MaterialsElectrocatalysts for Energy ConversionAdvanced Battery Technologies Research