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Integrating Mobile and Fixed-Site Black Carbon Measurements to Bridge Spatiotemporal Gaps in Urban Air Quality

Chirag Manchanda, Robert A. Harley, Julian Marshall, Alexander J. Turner, Joshua S. Apte

2024Environmental Science & Technology12 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide Urban air pollution can vary sharply in space and time. However, few monitoring strategies can concurrently resolve spatial and temporal variation at fine scales. Here, we present a new measurement-driven spatiotemporal modeling approach that transcends the individual limitations of two complementary sampling paradigms: mobile monitoring and fixed-site sensor networks. We develop, validate, and apply this model to predict black carbon (BC) using data from an intensive, 100-day field study in West Oakland, CA. Our spatiotemporal model exploits coherent spatial patterns derived from a multipollutant mobile monitoring campaign to fill spatial gaps in time-complete BC data from a low-cost sensor network. Our model performs well in reconstructing patterns at fine spatial and temporal resolution (30 m, 15 min), demonstrating strong out-of-sample correlations for both mobile (Pearson’s R ∼ 0.77) and fixed-site measurements ( R ∼ 0.95) while revealing features that are not effectively captured by a single monitoring approach in isolation. The model reveals sharp concentration gradients near major emission sources while capturing their temporal variability, offering valuable insights into pollution sources and dynamics.

Topics & Concepts

Sampling (signal processing)Temporal resolutionEnvironmental scienceAir quality indexField (mathematics)Computer scienceSpatial ecologySpatial variabilityEnvironmental monitoringRemote sensingSample (material)Wireless sensor networkData miningMeteorologyGeographyTelecommunicationsEcologyStatisticsEnvironmental engineeringPure mathematicsComputer networkPhysicsDetectorChemistryQuantum mechanicsMathematicsBiologyChromatographyAir Quality and Health ImpactsAir Quality Monitoring and ForecastingAtmospheric chemistry and aerosols
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