Mechanism of the selective catalytic reduction of NO<sub>x</sub> with CH<sub>4</sub> on In/H-beta
Jiuhu Zhao, Zhi Li, Rongshu Zhu, Jingwen Zhang, Ran Ding, Zhengzhong Wen, Yongji Zhu, Gaige Zhang, Baiyang Chen
Abstract
Firstly, CH<sub>4</sub> would be activated to CH<sub>3</sub>OH, subsequently, CH<sub>3</sub>OH and O* reacted to generate HCOO<sup>−</sup>. Finally, the HCOO<sup>−</sup> further reacted with NO<sub>3</sub><sup>−</sup> which was completely converted to CO<sub>2</sub>, H<sub>2</sub>O and N<sub>2</sub>.
Topics & Concepts
CatalysisChemistryCrystallographyStereochemistryPhysicsOrganic chemistryCatalytic Processes in Materials ScienceCatalysis and Oxidation ReactionsAmmonia Synthesis and Nitrogen Reduction