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Metal-oxide interface reactions and their effect on integrated resistive/threshold switching in NbO <i> <sub>x</sub> </i>

Shimul Kanti Nath, Sanjoy Kumar Nandi, Shuai Li, Robert Glen Elliman

2020Nanotechnology30 citationsDOIOpen Access PDF

Abstract

/Pt devices. In particular, devices are shown to exhibit stable threshold switching under negative bias but to have a response under positive bias that depends on the choice of metal. Three distinct responses are highlighted: Devices with Nb and Ti top electrodes are shown to exhibit stable threshold switching with symmetric characteristics for both positive and negative polarities; devices with Cr top electrodes are shown to exhibit stable threshold switching but with asymmetric hysteresis windows under positive and negative polarities; and devices with Ta and Hf electrodes are shown to exhibit an integrated threshold-memory (1S1M) response. Based on thermodynamic data and lumped element modelling these effects are attributed to the formation of a metal-oxide interlayer and its response to field-induced oxygen exchange. These results provide important insight into the physical origin of the switching response and pathways for engineering devices with reliable switching characteristics.

Topics & Concepts

Materials scienceHysteresisElectrodeOptoelectronicsFast switchingMetalOxygenThreshold voltageBiasingSwitching timeChemical physicsVoltageInterface (matter)Condensed matter physicsResponse timeNanotechnologyAdvanced Memory and Neural ComputingTransition Metal Oxide NanomaterialsFerroelectric and Negative Capacitance Devices