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Highly Biaxially Strained Silicene on Au(111)

Daniele Nazzari, Jakob Genser, Viktoria Ritter, Ole Bethge, E. Bertagnolli, Georg Ramer, Bernhard Lendl, Kenji Watanabe, Takashi Taniguchi, Riccardo Rurali, Miroslav Kolı́bal, Alois Lugstein

2021The Journal of Physical Chemistry C20 citationsDOIOpen Access PDF

Abstract

investigation, we passivated the silicene on Au(111) by encapsulating it under few layers hBN or graphene flakes. The observed spectrum is characterized by vibrational modes that are strongly red-shifted with respect to the ones expected for freestanding silicene. By comparing low-energy electron diffraction (LEED) patterns and Raman results with first-principles calculations, we show that the vibrational modes indicate a highly (>7%) biaxially strained silicene phase.

Topics & Concepts

SiliceneMaterials scienceRaman spectroscopyGrapheneMonolayerCondensed matter physicsBrillouin zoneBand gapSiliconElectron diffractionNanotechnologyOptoelectronicsDiffractionOpticsPhysicsGraphene research and applicationsTopological Materials and PhenomenaQuantum and electron transport phenomena
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