Spin-photogalvanic effect in chiral lead halide perovskites
Ruiheng Pan, Xiantong Tang, Lixuan Kan, Yang Li, Haomiao Yu, Kai Wang
Abstract
polycrystalline film-based lateral devices (100 μm channel length). The light helicity dependence of the short-circuit photocurrent exhibits the circular photogalvanic effect (CPGE) and linear photogalvanic effect (LPGE) with decent two-fold symmetry for a complete cycle in a wide temperature range from 4 K to 300 K. Because of the Rashba SOC and the material helicity, the effect is converse for the two chiral LHPs. In addition, its magnitude and sign can be effectively tuned by constant magnetic fields. The Rashba effect, CISS-generated unbalanced spin transport, and chiral-induced magnetization are mutually responsible for it. Our study evidently proves the future prospect of using chiral LHPs for spin-orbitronics.