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Increased carbon capture by a silicate-treated forested watershed affected by acid deposition

Lyla L. Taylor, Charles T. Driscoll, Peter M. Groffman, Greg H. Rau, Joel D. Blum, David J. Beerling

2021Biogeosciences91 citationsDOIOpen Access PDF

Abstract

Abstract. Meeting internationally agreed-upon climate targets requires carbon dioxide removal (CDR) strategies coupled with an urgent phase-down of fossil fuel emissions. However, the efficacy and wider impacts of CDR are poorly understood. Enhanced rock weathering (ERW) is a land-based CDR strategy requiring large-scale field trials. Here we show that a low 3.44 t ha−1 wollastonite treatment in an 11.8 ha acid-rain-impacted forested watershed in New Hampshire, USA, led to cumulative carbon capture by carbonic acid weathering of 0.025–0.13 t CO2 ha−1 over 15 years. Despite a 0.8–2.4 t CO2 ha−1 logistical carbon penalty from mining, grinding, transportation, and spreading, by 2015 weathering together with increased forest productivity led to net CDR of 8.5–11.5 t CO2 ha−1. Our results demonstrate that ERW may be an effective, scalable CDR strategy for acid-impacted forests but at large scales requires sustainable sources of silicate rock dust.

Topics & Concepts

WeatheringWatershedEnvironmental scienceCarbon dioxideCarbon sequestrationCarbonic acidCarbon cycleSilicateCarbon fibersDeposition (geology)Carbon sinkHydrology (agriculture)GeologyClimate changeGeochemistryChemistryEcosystemSedimentMaterials scienceGeomorphologyEcologyBiologyPhysical chemistryComposite materialOrganic chemistryComputer scienceMachine learningComposite numberOceanographyGeotechnical engineeringCO2 Sequestration and Geologic InteractionsMine drainage and remediation techniquesGeological and Geophysical Studies Worldwide
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