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Electrochemical Oxidative Dehydrogenative Coupling of Sulfoximines to Construct N‐sulfenyl and N‐phosphinyl Sulfoximines

Xiaoman Li, Jiawei Huang, Liang Xu, Jichang Liu, Yu Wei

2023Advanced Synthesis & Catalysis18 citationsDOI

Abstract

Abstract Herein, an electrochemical oxidative approach for the synthesis of N‐sulfenyl and N‐phosphinyl sulfoximines has been established from readily available NH‐sulfoximines with thiophenols and diarylphosphine oxides. Utilizing the synergistic effect of halide salt and electrochemical oxidation, the desired products are obtained at room temperature in the absence of any acidic/basic/metallic additives.

Topics & Concepts

ChemistryElectrochemistryHalideOxidative phosphorylationCoupling (piping)Salt (chemistry)Combinatorial chemistryOrganic chemistryElectrodeMetallurgyPhysical chemistryBiochemistryMaterials scienceSynthesis and Catalytic ReactionsCatalytic C–H Functionalization MethodsSulfur-Based Synthesis Techniques