Regulating the electronic structure of metal–organic frameworks <i>via</i> ion-exchanged Ir dispersion for robust overall water splitting
Shunfa Zhou, Yuxuan Liu, Jiawei Shi, Jing‐Feng Li, Weiwei Cai
Abstract
A facile ion exchange strategy to fabricate CoIr x –BDC with atomically dispersed Ir, which requires only 9 and 80 mV to deliver 10 and 100 mA cm −2 HER, respectively, and only 245 mV to reach 100 mA cm −2 OER.
Topics & Concepts
Water splittingDispersion (optics)IonIon exchangeMetal-organic frameworkMaterials scienceMetalChemistryNanotechnologyInorganic chemistryCatalysisPhysical chemistryOpticsPhysicsMetallurgyOrganic chemistryPhotocatalysisAdsorptionElectrocatalysts for Energy ConversionMetal-Organic Frameworks: Synthesis and ApplicationsAdvanced Memory and Neural Computing