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Potentiometric Performance of Ion-Selective Electrodes Based on Polyaniline and Chelating Agents: Detection of Fe2+ or Fe3+ Ions

Rimeh Ismail, Ivana Šeděnková, Zulfiya Černochová, Iryna Romanenko, Ognen Pop‐Georgievski, Martin Hrubý, Elena Tomšík

2022Biosensors17 citationsDOIOpen Access PDF

Abstract

We constructed a sensor for the determination of Fe2+ and/or Fe3+ ions that consists of a polyaniline layer as an ion-to-electron transducer; on top of it, chelating molecules are deposited (which can selectively chelate specific ions) and protected with a non-biofouling poly(2-methyl-2-oxazoline)s layer. We have shown that our potentiometric sensing layers show a rapid response to the presence of Fe2+ or Fe3+ ions, do not experience interference with other ions (such as Cu2+), and work in a biological environment in the presence of bovine serum albumin (as a model serum protein). The sensing layers detect iron ions in the concentration range from 5 nM to 50 µM.

Topics & Concepts

Potentiometric titrationChelationIonPolyanilineChemistryElectrodeIon selective electrodeInorganic chemistryMoleculeBovine serum albuminAnalytical Chemistry (journal)ChromatographySelectivityPolymerOrganic chemistryPhysical chemistryPolymerizationCatalysisAnalytical Chemistry and SensorsElectrochemical sensors and biosensorsConducting polymers and applications
Potentiometric Performance of Ion-Selective Electrodes Based on Polyaniline and Chelating Agents: Detection of Fe2+ or Fe3+ Ions | Litcius